Nonlinear molecular spectroscopy ================================ Sum-of-states (SOS) for multilevel system ------------------- Computationally cheap and intuitive. .. note:: In the SOS method, dissipation and decoherence are introduced phenomelogically. Correlation function approach ----------------------------- Direct computing the many-point correlation functions with the quantum regression theorem * Closed quantum systems * Open quantum systems Valid for open quantum systems where environment effects can be rigirously described with quantum master equations. Visulize with double-sided Feynman diagrams instead of the time-loop diagrams. * Many-body systems Solve Dyson equaiton for one-particle Green's function .. math:: G = G_0 + G_0 \Sigma G Non-perturbative approah ------------------------- valid for ALL systems if a quantum dynamics solver is provided. Simulating the laser-driven dynamics including explicitly all laser pulses. This usually requires phase clcyling to remove unwanted pathways.